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Ultrafast Defect Manipulation with Optical Anisotropy in Fused Silica

Published online by Cambridge University Press:  31 January 2011

Yasuhiko Shimotsuma ,
Masaaki Sakakura ,
Peter G. Kazansky ,
Kiyotaka Miura  and
Kazuyuki Hirao
Yasuhiko Shimotsuma
Affiliation:
yshimotsu@yahoo.co.jpyshimo@collon1.kuic.kyoto-u.ac.jp
Masaaki Sakakura
Affiliation:
masa@collon1.kuic.kyoto-u.ac.jp, Kyoto University, Innovative Collaboration Center, Kyoto, Japan
Peter G. Kazansky
Affiliation:
pgk@orc.soton.ac.uk, University of Southampton, Optoelectronics Research Centre, Southampton, United Kingdom
Kiyotaka Miura
Affiliation:
kmiura@collon1.kuic.kyoto-u.ac.jp, Kyoto University, Department of Material Chemistry, Kyoto, Japan
Kazuyuki Hirao
Affiliation:
hirao@bisco1.kuic.kyoto-u.ac.jp, Kyoto University, Department of Material Chemistry, Kyoto, Japan
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Abstract

We report the evidence that the oxygen defects induced by focusing an intense infrared femtosecond laser pulse in fused silica can be self-organized by the interference pattern between photon and electron plasma wave. Self-organized nanostructure with a sub-wavelength modulation in refractive index exhibits form birefringence which is rewritable and directionally-controllable. Intriguingly, such optical anisotropy, which indicates a remarkable non-reciprocity, has initially evolved from residual birefringence originated from internal stress distribution due to local heating followed by structural change, regardless of interpulse time. This anisotropic light-matter interaction could be interpreted in terms of an asymmetric relation between light polarization and pulse front tilt. Apart from fundamental understanding of self-organization mechanism, the direction of encoded birefringence can introduce an entirely new concept for rewritable optical storage beyond the diffraction limit of light.

Keywords

lasernanostructureamorphous
Type
Research Article
Information
MRS Online Proceedings Library (OPL) , Volume 1230: Symposium MM – Ultrafast Processes in Materials Science , 2009 , 1230-MM07-05
Copyright
Copyright © Materials Research Society 2010

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