Hostname: page-component-cd9895bd7-gvvz8 Total loading time: 0 Render date: 2024-12-29T10:13:02.735Z Has data issue: false hasContentIssue false

Measuring 14C Concentration in Wine to Monitor Global Distribution of 14C

Published online by Cambridge University Press:  09 February 2016

Hirohisa Sakurai*
Affiliation:
Department of Physics, Yamagata University, Yamagata, Japan
Saori Namai
Affiliation:
Graduate School of Science and Engineering, Yamagata University, Yamagata, Japan
Emiko Inui
Affiliation:
Faculty of Science, R.I. Laboratory, Yamagata University, Yamagata, Japan
Fuyuki Tokanai
Affiliation:
Department of Physics, Yamagata University, Yamagata, Japan
Kazuhiro Kato
Affiliation:
Faculty of Science, Yamagata University, Yamagata, Japan
Yui Takahashi
Affiliation:
Graduate School of Science and Engineering, Yamagata University, Yamagata, Japan
Taichi Sato
Affiliation:
Graduate School of Science and Engineering, Yamagata University, Yamagata, Japan
Satoshi Kikuchi
Affiliation:
Fujitsu Ltd., Numazu, Japan
Yumi Arai
Affiliation:
Department of Physics, Yamagata University, Yamagata, Japan
Kimiaki Masuda
Affiliation:
STE Lab, Nagoya University, Nagoya, Japan
Katsumasa Shibata
Affiliation:
Graduate School of Science and Engineering, Yamagata University, Yamagata, Japan
Yasunao Kuriyama
Affiliation:
Department of Material and Biological Chemistry, Yamagata University, Yamagata, Japan
*
2Corresponding author. Email: sakurai@sci.kj.yamagata-u.ac.jp.

Abstract

Using liquid scintillation counting (LSC) and accelerator mass spectrometry (AMS), radiocarbon concentrations were measured for wine from 8 wineries located in 7 countries in the Northern and Southern hemispheres. The 14C concentrations of ethanol and residual materials in the wine were correlated (correlation coefficient 0.82). The δ14C measurements of wine samples from the mid-latitudes in the Northern Hemisphere were approximately 1l% lower than the extrapolations from Schauinsland data, suggesting a local fossil fuel effect. δ14C measurements from the wine samples from the Southern Hemisphere were higher than those from the Northern Hemisphere. The offsets of the 4 wine δ14C measurements were significant, with values between approximately 8% and 15%. Because the harvest years of the mixed grapes were estimated to be 7–12 yr older than their vintage years, this leads to a caveat when determining the 14C concentrations of the year using the wine vintage.

Type
Unusual Applications of 14C Measurement
Copyright
Copyright © 2013 by the Arizona Board of Regents on behalf of the University of Arizona 

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

Beer, J, McCracken, K, von Steiger, R. 2012. Cosmogenic Radionuclides. Berlin: Springer.CrossRefGoogle Scholar
Burchuladze, AA, Pagava, SV, Povinec, P, Togonidze, GI, Usacev, S. 1980. Radiocarbon variations with the 11-year solar cycle during the last century. Nature 287(5780):320–2.CrossRefGoogle Scholar
Burchuladze, AA, Chudy, M, Eristavi, IV, Pagava, SV, Povinec, P, Sivo, A, Togonidze, GI. 1989. Anthropogenic 14C variations in atmospheric CO2 and wines. Radiocarbon 31(3):771–6.CrossRefGoogle Scholar
Ehleringer, JR, Casale, JF, Barnette, JE, Xu, X, Lott, MJ. 2011. 14C calibration curves for modern plant material from tropical regions of South America. Radiocarbon 53(4):585–94.CrossRefGoogle Scholar
Hua, Q, Barbetti, M. 2004. Review of tropospheric bomb 14C data for carbon cycle modeling and age calibration purposes. Radiocarbon 46(3):1273–98.CrossRefGoogle Scholar
Levin, I, Kromer, B. 2004. The tropospheric 14CO2 level in mid-latitudes of the Northern Hemisphere (1959–2003). Radiocarbon 46(3):1261–72.CrossRefGoogle Scholar
Nydal, R. 1968. Further investigation on the transfer of radiocarbon in nature. Journal of Geophysical Research 73(12):3617–35.CrossRefGoogle Scholar
Nydal, R, Lovseth, K. 1983. Tracing bomb 14C in the atmosphere 1962–1980. Journal of Geophysical Research 88:3621–42.CrossRefGoogle Scholar
Palstra, SWL, Karstens, U, Streurman, HJ, Meijer, HAJ. 2008. Wine ethanol 14C as a tracer for fossil fuel CO2 emissions in Europe: measurements and model comparison. Journal of Geophysical Research 113: D21305, doi:10.1029/2008JD010282.CrossRefGoogle Scholar
Rakowski, AZ, Nakamura, T, Pazdur, A. 2008. Variations of anthropogenic CO2 in urban area deduced by radiocarbon concentration in modern tree rings. Journal of Environmental Radioactivity 99(10):1558–65.CrossRefGoogle ScholarPubMed
Sakurai, H, Tokanai, F, Kato, K, Takahashi, Y, Sato, T, Masuda, K, Miyahara, H, Mundia, C, Tavera, W. 2013. Latest 14C concentrations of plant leaves at high altitudes in the Northern and Southern hemispheres: vertical stability of local suess effect. Radiocarbon, these proceedings, doi:10.2458/azu_is_rc.55.16273.CrossRefGoogle Scholar
Schönhofer, F. 1992. 14C in Austrian wine and vinegar. Radiocarbon 34(3):768–71.CrossRefGoogle Scholar
Takahashi, Y, Sakurai, H, Inui, E, Namai, S, Sato, T. 2011. Radiocarbon measurement of biodiesel fuel using the liquid scintillation counter Quantulus. In: Cassette, P, editor. LSC 2010, Advances in Liquid Scintillation Spectrometry. Tucson: Radiocarbon. p 41–6.Google Scholar
Tokanai, F, Kato, K, Anshita, M, Izumi, A, Sakurai, H, Saito, T. Compact AMS system at Yamagata University. AIP Conference Proceedings 1336:70–4.Google Scholar