In our earlier papers, we demonstrated that plasma pressure decreases with the growing atomic number of the target material. That experimentally confirmed fact brought about a question whether it would be possible to collimate the Al plasma outflow by using plastic plasma as a compressor. To prove that idea we used in our next experiments a plastic target with an Al cylindrical insert of 400 µm in diameter. The measurements were carried out at the Prague Asterix Laser System iodine laser facility. The laser provided a 250 ps (full width at half maximum (FWHM)) pulse with energy of 130 J at the third harmonic frequency (λ3 = 0.438 µm). The focal spot diameters (ΦL) 800, 1000, and 1200 µm ensured predominance of the plastic plasma amount high enough for the effective Al plasma compression. To study the Al plasma stream propagation and its interaction with plastic plasma a three-frame interferometric system and an X-ray camera were used. The experiment provided a proof that creation of the collimated Al plasma jet by action of outer plastic plasma is feasible. In order to discuss of the experimental results a thorough theoretical analysis was carried out.

Recent experimental results demonstrated that well formed plasma jets can be produced at laser interaction with targets made of materials with high atomic number (A ≥ 29 where A = 29 corresponds to Cu). On the contrary, it is impossible to launch a plasma jet on low-A material targets like plastic. This paper is aimed at explanation of this difference by considering mechanisms responsible for plasma jet formation, i.e., the radiative cooling of ablative plasma and the influence of target irradiation annular profile speculated hitherto, newly complemented by different expansion regimes of the Cu and plastic plasmas (provided by numerical simulations). The experiment was carried out with the PALS iodine laser. Two different planar massive targets, plastic and Cu, as well as the plastic target covered by thin Cu layers of various thicknesses were irradiated by the third harmonic laser beam of energy of 30 J, pulse duration of 250 ps (full width at half maximum), and the focal spot radius of 400 µm. To find the most suitable range of these layers (from 28 to 190 nm) a simple analytical model of laser-driven evaporation was developed. Three-frame laser interferometer and an X-ray streak camera were used as two main diagnostic tools. Numerical modeling was performed with the use of two-dimensional hydrodynamic code ATLANT-HE. Results provided from experiments and theoretical analyses have proved that the process of plasma jet formation is rather complex. Relative importance of the three mechanisms mentioned above depends on the target irradiation geometry as well as the target material used.

Quantitative EPMA (electron probe microanalysis) intensity measurements require an accurate correction for the X-ray continuum (or background) created by the Bremsstrahlung effect from the primary electron beam. This X-ray continuum, as measured on a wavelength-dispersive spectrometer at any particular wavelength, is primarily a function of the mean atomic number of the material being analyzed. One can calibrate the dependence of the continuum on mean atomic number by measuring and curve fitting the X-ray intensities at the analytical peak in pure elements, oxides, and binary compound standards that do not contain any of the analyte or any interfering elements and use that calibration to calculate the X-ray background correction. For unknown samples, the mean atomic number is determined from the elemental concentrations calculated by the ZAF or φ(ρz) matrix correction, and the fit regression coefficients are used iteratively to calculate the actual background correction. Over a large range of mean atomic number we find that the dependence of the continuum intensity on mean atomic number is well described by a second-order polynomial fit. In the case of low-energy X-ray lines (<1 to 2 keV), this fit is significantly improved by correcting the X-ray continuum intensities for absorption. For major and most minor element analyses, the improved mean atomic number background correction procedure presented in this paper is accurate and robust for a wide variety of samples. Empirical mean atomic number background data are presented for a typical 10-element silicate and a 15-element sulfide analytical set up that demonstrate the validity of the technique as well as some potential limitations.