The rotational joint plays a vital role in the industrial and civil areas, which is typically utilized to achieve the relative rotation between the adjacent parts. Generally, structuring a conventional rotational joint involves the bulk actuators (e.g., motor and hydraulic cylinders) and complex structures, bringing difficulty for miniaturing the dimension. In this paper, a class of novel rotational mechanisms, which were constructed by the combination of compliant mechanisms (e.g., cartwheel pivot and multileaf pivot) and intelligent actuator (e.g., shape memory alloy (SMA) wire and spring), was proposed to reduce the complexity of the conventional rotational joints. As the case study, a novel SMA wire-driven flexural rotational mechanism (SDFRM), which is constructed by the cartwheel pivot and SMA wire, was developed to demonstrate the feasibility of combining the compliant mechanism and smart actuator. After establishing the static model of the cartwheel pivot and the thermal effect model of the SMA wire, the overall model of SDFRM was developed for the comprehensive performance analysis and the control system design. After that, the model validation and experiments were performed with the proposed prototype and control system. It can be seen from the experimental results that the proposed model can be validated within the error of 3.8%. In addition, the performance study on SDFRM indicates that the prototyped SDFRM system can track the given trajectories within the error of 0.2 mm in the workspace. As a result, the proposed concept was demonstrated as an effective way to reduce the dimension and weight of the conventional rotational joint.