Motivated by the achieved high intensities of novel extreme ultraviolet (XUV) radiation sources, such as free electron lasers and laser-driven high harmonic generation beamlines, we elaborate on their perspective in inducing observable strong field effects. The feasibility of extending such effects from the infrared and visible spectral regimes in the XUV domain is supported through numerically calculated models of near-future experiments. We highlight the advancement of performing studies in the time domain, using ultra-short XUV pulses, which allows for the temporal evolution of such effects to be followed. Experimental and theoretical obstacles and limitations are further discussed.

The generation of high-order harmonics in ultraviolet spectral range by targets of periodic modulation interacting with relativistic, high contrast laser pulse (Iλ2 = 1020 W/cm2 · μm2) was investigated experimentally and numerically. The spectral intensity of the 2nd- and 3rd-order harmonic emission from grating of different periodicities (250, 410, and 480 nm) is presented. The enhancement of the 3rd harmonic order compared with 2nd was observed for a grating of 480 nm periodicity. The experimental results indicate the role of the grating periodicity on the emission efficiency of different higher order harmonics in the UV spectral range. The higher order harmonics are emitted at the grating surface separated from the specular reflection of the laser pulse, due of the interference effects. In addition, 2D numerical PIC simulations demonstrate a complex angular distribution of the higher harmonics (HH) spectral intensity and confirm the strong dependence of the HH efficiency of a specific order on the grating periodicity, as observed experimentally. These special features of the high harmonic emission by periodically modulated targets open the route toward the control of HH spectral composition and of the emission efficiency of the lower order harmonics.

Optical vortices are structures of the electromagnetic field with a spiral phase ramp about a point-phase singularity, carrying orbital angular momentum (OAM). Recently, OAM has been imprinted to short-wavelength radiation through high-order harmonic generation (HHG), leading to the emission of attosecond twisted beams in the extreme-ultraviolet (XUV) regime. We explore the details of the mapping of the driving vortex to its harmonic spectrum. In particular, we show that the geometry of the harmonic vortices is convoluted, arising from the superposition of the contribution from the short and long quantum paths responsible of HHG. Finally, we show how to take advantage of transverse phase-matching to select twisted attosecond beams with different spatiotemporal properties.

Intense laser light incident on solid targets has been shown to be a prolific source of harmonics. High harmonic intensities are characterized by a power-law spectrum Pm~m−p, where p denotes a spectral decay index and m is the harmonic number. Across a wide range of light intensity and target plasma density, particle-in-cell (PIC) simulations have shown p = 8/3, a value supported by the observation. However, the claim that this decay is universal has been contested and shown to break down in simulations when the incident light is P-polarized. Here weaker decays with p = 5/3 and at higher intensities p = 4/3 were observed. The distinction between the two regimes was attributed to the contribution to the spectrum from emission at the plasma frequency and its harmonics from Langmuir waves excited by the Brunel electrons generated when the incident light is P-polarized. In the present work, a single-particle model has been devised to lend support to a wide range of PIC data. The model incorporates a Langmuir electric field and is hybrid in the sense that we have made use of PIC output to guide our choice of field amplitudes in the Langmuir source. We find that the spectrum computed in this way shows generally satisfactory agreement with the corresponding PIC spectra, both in decay coefficient and spectral cut-off. At the highest intensities considered the emission from the convective bunching of electrons in high-amplitude Langmuir waves is itself superseded by Brunel electron bremsstrahlung and we have identified the regions of parameter space over which each of these sources is dominant. Interestingly, the same distinction has been drawn in a very different plasma regime where comparably complex spectra have been predicted in gamma-ray burst spectra from Langmuir turbulence produced in astrophysical jets.

High harmonic generation in gas jets was investigated in different gases up to more than 14 bar backing pressure. The observation of increase of harmonic intensity with increasing pressure and laser intensity shows evidence of the presence of clusters in Xe with an increased efficiency compared with He, whereas Ar is an intermediate case for which clusters will start to dominate above a certain backing pressure. Spectral investigations give evidence for tunable harmonic generation in a broad spectral range. A spectral shift of opposite signature caused by the free electrons in the focal volume and the nanoplasmas inside the cluster was observed.

We study the generation of high-order harmonics from plasma plume, by using the 20 TW, 10 Hz laser of the Advanced Laser Light Source (ALLS). We perform detailed studies on enhancement of single high-order harmonics generated in laser plasma using the fundamental and second harmonic of the ALLS beam line. Quasi-monochromatic harmonics are observed for Mn, Cr, Sb, Sn, and In plasmas. We identify most of the ionic/neutral transitions responsible for the enhancement, which all have strong oscillator strengths. Intensity enhancements of the 13th, 17th, 21st, 29th, and 33rd harmonics from these targets are demonstrated using the 800 nm pump laser and varying its chirp. We also observed harmonic enhancement from some targets for 400 nm pump laser. Using Mn plume, we demonstrated the highest harmonic photon energy (52.9 eV) at which enhancement has been observed (17th order, λ = 23.5 nm).

We perform systematic investigation of a new method for generating high-order harmonics, using ablation as the nonlinear medium. We place emphasis on clarifying the pump laser conditions for optimum harmonic yield. For this purpose, we use the Ti:Sapphire laser beams of the advanced laser light source (800 nm wavelength, 360 mJ total energy). We have independently varied the intensity of the prepulse (which creates the plasma ablation) and the intensity of the main pulse (which generates the harmonics), and studied their influence on the harmonic intensity. We show here that the presence of doubly ionized atoms in the ablation, created either by a strong prepulse intensity or by irradiating the main pulse, will suppress harmonic generation.