Very good absorption of ultra short laser pulses by clusters is a well
established fact. Efficient collisional absorption occurs only in the
initial phase of the pulse. However, experiments and numerical simulations
show that even after collisional absorption becomes inefficient subsequent
to heating of the electrons, strong absorption continues. There have been
a few attempts to model this phenomenon in terms of driven
“linear” oscillator models with time dependent
eigen-frequencies. Here we propose a nonlinear oscillator model and show
that nonlinear resonance is the leading mechanism responsible for the
collisionless absorption. Further it is demonstrated, on the basis of
Lyapunov spectra, that laser-cluster interaction, under certain
conditions, exhibits chaotic behavior.