Rabindranath Tagore's visit to China in 1924 was a milestone in the May Fourth Movement's envisioning of modern literature as a vehicle for social transformation. Moving beyond interpretations of the visit as a political failure, this article locates the reception of Tagore's ideal of Eastern spirituality within the larger climate of literary production, specifically in new poetry. Through close reading of poems by Xu Zhimo and Bing Xin, this article argues that Tagore's ideas were fundamental for the development of poetry as an interpersonal medium that both portrays and effects social bonds. This understanding developed as Chinese poets and literary critics engaged with Tagore's critique of Western materialism and his positioning of Asian religious sensibilities in contrast to Western materialism. Tagore's view promoted literature as a medium connecting religion, the individual, and the universe. In this sense, though Tagore's pan-Asianism failed as a viable political project, it carried powerful resonance in the arena of modern Chinese literature.