Fluvial and colluvial deposits of Late Holocene age in South-Central Ontario catchments have provided few 14C dates, most by conventional methods registering century-old ages. Other young deposits, dated by conventional and accelerator mass spectrometry radiocarbon (AMS 14C), have yielded bomb-affected post-1950 ages over variable time limits. Attempts to date the base of Ah and lower-in-section soil horizons, in Early to Late Holocene stream terrace deposits, have yielded atomic bomb effects. Comparing bomb contamination in Late Holocene fluvial deposits, using both conventional and AMS methods, identifies a mix of bomb-affected beds juxtaposed with dated beds, the latter yielding ages with narrow standard deviations. Colluvial deposits overlying key glacial sections in the Rouge Catchment, while rare, yield bracketed AMS ages for an Ahbk horizon that refines weathering times relative to previously obtained conventional 14C dates. Bomb-affected sediment appears variably distributed within floodplain soils and in the ground soil of a colluvial section. Mass wasted deposits, with AMS 14C ages spread over the last few centuries, appear related to Little Ice Age (LIA) changes in climate, corroborated by pollen records. Further, these AMS-14C dated beds calibrate weathering of secondary Fe-Al oxihydroxides over the first half a millennium of weathering time.