Spectral observations show that volcanic glass is the dominant ingredient of the aeolian landforms which cover the northern lowlands on Mars. Surface winds subject these sands to physical alteration processes in the present-day surface environment. This work highlights the role of glaciovolcanism throughout Mars’ geologic history and the parallels with landforms and materials found in Iceland. As the physical properties of Martian volcanic glass particles are difficult to constrain from orbit, Icelandic materials can provide valuable insights in their transport and modification characteristics. The processing of glass grains by environmental processes by means of the dune transport cycle is discussed. Experiments targeted the grain-size alteration effects experienced during the dune transport cycle, including the effect of ‘low-energy’ avalanching and ‘high-energy’ aeolian regimes (i.e. particle rolling and saltation). Saltation transport was found to rapidly alter grains and particle size distributions, which contributes to a positive feedback loop where the new smaller grains are mobilised more easily after fracturing and surficial abrasion. Post-depositional physical alteration therefore needs to be reconciled with the present-day silicic spectral signatures of these glasses in order to infer the relevant landform genetic. This effort is especially relevant in respect to the loss of possible signatures of biochemical alteration from microbial interactions, as glaciovolcanic environments are favourable habitats for life. As chemical and physical weathering is limited to the grain exterior, the grain interior may still retain a geochemical record of the subglacial eruption environment in which these grains were formed. Quantification of the volatiles sequestered in the glass can therefore be used to identify the formative conditions of the amorphous component in aeolian sediments.