In this paper, we innovatively conduct a Porro prism-based beam pointing stability promotion technique research and realize a high-performance rod-type photonic crystal fiber-based chirped pulse amplification (CPA) system, mainly including a frequency-reduced all-fiber pre-amplification stage, photonic crystal rod-based main amplification stage, and 1600 lines/mm transmission grating-pair compressor. Laser output with average power of 50 W, repetition rates of 500 kHz, pulse energy of 100 μJ, pulse duration of 830 fs, beam quality of M2<1.3, power fluctuation of 0.55% root mean square, and beam pointing drift of 19 μrad/°C over 8 h is realized. The high-performance laser system has an enormous application potential in fundamental research and precision manufacturing fields.

The dispersion of a pair of prisms is analyzed by means of a ray-tracing method operating at other than tip-to-tip propagation of the prisms, taking into consideration the limited spectral bandwidth. The variations of the group delay dispersion and the third-order dispersion for a pair of prisms are calculated with respect to the incident position and the separation between the prisms. The pair of prisms can provide a wide range of independent and continuous third-order dispersion compensation. The effect of residual third-order dispersion on the pulse contrast ratio and pulse duration is also calculated. The residual third-order dispersion not only worsens the pulse contrast ratio, but also increases the pulse duration to the hundreds of femtosecond range for a tens of femtosecond pulse, even when the residual third-order dispersion is small. These phenomena are helpful in compensating for the residual high-order dispersion and in understanding its effect on pulse contrast ratios and pulse durations in ultrashort laser systems.

High harmonic generation in gas jets was investigated in different gases up to more than 14 bar backing pressure. The observation of increase of harmonic intensity with increasing pressure and laser intensity shows evidence of the presence of clusters in Xe with an increased efficiency compared with He, whereas Ar is an intermediate case for which clusters will start to dominate above a certain backing pressure. Spectral investigations give evidence for tunable harmonic generation in a broad spectral range. A spectral shift of opposite signature caused by the free electrons in the focal volume and the nanoplasmas inside the cluster was observed.