Hostname: page-component-cd9895bd7-mkpzs Total loading time: 0 Render date: 2024-12-27T12:56:43.424Z Has data issue: false hasContentIssue false

Emission spectra of noble gases and their mixtures under ion beam excitation

Published online by Cambridge University Press:  17 October 2016

M.U. Khasenov*
Affiliation:
National Laboratory Astana, Nazarbayev University, 53 Kabanbay Batyr Avenue, Astana 010000, Kazakhstan
*
Address correspondence and reprint requests to: M.U. Khasenov, National Laboratory Astana, Nazarbayev University, 53, Kabanbay Batyr Avenue, NLA, Astana 010000, Kazakhstan. E-mail: mendykhan.khassenov@nu.edu.kz

Abstract

The luminescence spectra of noble gases and their binary mixtures were measured using heavy ion beam excitation from a DC-60 accelerator. Spectra were measured in the range of 200–975 nm; the gas spectra were dominated by lines of ps and dp atomic transitions; in neon and argon, lines from atomic oxygen, N2, N2 +, and OH radical bands were also observed. The ultraviolet region of the spectra was represented by a “third continuum” of noble gases. In krypton, the band of the KrO excimer molecule with a maximum at 557 nm was also observed. The maxima of the heteronuclear ionic molecules bands were located at wavelengths of 329 and 506 nm (Ar–Xe), 491 nm (Kr–Xe), and 642 nm (Ar–Kr). The relative intensities of the 2p–1s transitions of the noble gases atoms were measured and are discussed.

Type
Research Article
Copyright
Copyright © Cambridge University Press 2016 

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

REFERENCES

Abramov, A.A., Gorbunov, V.V., Melnikov, S.P., Mukhamatullin, A.Kh., Pikulev, A.A., Sinitsyn, A.V., Sinyanskii, A.A. & Tsvetkov, V.M. (2006). Luminescence of nuclear-induced rare-gas plasmas in near infrared spectral range. Proc. SPIE 6263, 279296.Google Scholar
Bennett, W.R. (1962). Optical spectra excited in high pressure noble gases by alpha impact. Ann. Phys. 18, 367420.Google Scholar
Boichenko, A.M., Tarasenko, V.F., Fomin, E.A. & Yakovlenko, S.I. (1993). Broadband emission continua in rare gases and in mixtures of rare gases with halides. Quantum Electron. 23, 325.Google Scholar
Boichenko, A. M., Tarasenko, V. F. & Yakovlenko, S. I. (1999). The nature of third continua in rare gases. Laser Phys. 9, 10041020.Google Scholar
Boody, F.P. & Prelas, M.A. (1993). Absolutely calibrated spectra of nuclear-driven rare gases, 400–950 nm. Proc. Specialist Conf. “The Physics of Nuclear-Excited Plasma and the problems of Nuclear-Excited Lasers”, Vol. 2, pp. 149–155. Obninsk, Russia.Google Scholar
De Young, R.J. & Weaver, W.R. (1980). Spectra from nuclear-excited plasmas. J. Opt. Soc. Am. 70, 500506.Google Scholar
Friedl, W. (1959). Krypton-Xenon Banden. Z. Naturforsch. 14A, 848848a.Google Scholar
Gikal, B., Dmitriev, S., Apel, P., Bogomolov, S., Borisov, O., Buzmakov, V., Gulbekyan, G., Ivanenko, I., Ivanov, O., Itkis, M., Kazarinov, N., Kalagin, I., Kolesov, I., Papash, A., Paschenko, S., Tikhomirov, A. & Khabarov, M. (2008). DC-60 heavy ion cyclotron complex: The first beams and project parameters. Phys. Part. Nucl. Lett. 5, 642644.Google Scholar
Gorbunov, V.V., Grigor'ev, V.D., Dovbysh, L.E., Mel'nikov, S.P., Sinitsyn, A.V., Sinjanskii, A.A. & Tsvetkov, V.M. (2004). The luminescence spectra in the 350–875 nm range of the dense gas excited by uranium fission fragments. Proc. RFNC-VNIIEF, Issue 6, pp. 148–173 (in Russian).Google Scholar
Griegel, T., Drotleff, H.W., Hammer, J.W. & Petkau, K. (1990). The third continuum of the rare gases emitted by heavy ion beam induced plasmas. J. Chem. Phys. 93, 45814588.CrossRefGoogle Scholar
Ivanov, V.A. (1992). Dissociative recombination of molecular ions in noble-gas plasmas. Sov. Phys. – Usp. 35, 1736.CrossRefGoogle Scholar
Khasenov, M.U. (2005). Emission of ionic molecules (KrXe)+ at excitation by a hard ionizer. J. Appl. Spectrosc. 72, 316320.Google Scholar
Khasenov, M.U. (2006). Emission of the heteronuclear ionic molecules (ArXe)+ at excitation by a hard ionizer. Proc. SPIE 6263, 141148.Google Scholar
Khasenov, M.U. (2014). Mechanisms of population of the levels in gas lasers pumped by ionizing radiation. Laser Part. Beams 32, 501508.CrossRefGoogle Scholar
Kugler, E. (1964). Über die Lumineszenze der Edelgasgemische Ar/Xe, Kr/Xe, Ar/Kr und der Gemische Xe/N2 und Kr/N2 bei Angerung mit schnellen Elektronen. Ann. Phys., Leipzig 14, 137146.Google Scholar
Laigle, C. & Collier, F. (1983). Kinetic study of (ArXe)+ heteronuclear ion in electron beam excited Ar–Xe mixture. J. Phys. Ser. B 16, 687697.CrossRefGoogle Scholar
McCusker, M. (1984). The rare gas excimers. In Excimer Lasers. 2nd edn. (Rhodes, C.K., Ed.), pp. 4786. Berlin: Springer-Verlag.Google Scholar
Mel'nikov, S.P., Sizov, A.N., Sinyanskii, A.A. & Miley, G.H. (2015). Lasers with Nuclear Pumping. Heidelberg: Springer.Google Scholar
Millet, P., Barrie, A.M., Birot, A., Brunet, H., Dijols, H., Galy, G. & Salamero, J. (1981). Kinetic study of (ArKr)+ and (ArXe)+ heteronuclear ion emissions. J. Phys., Ser. B 14, 459472.Google Scholar
Mis'kevich, A.I. (1991). Visible and near-infrared direct nuclear pumped lasers. Laser Phys. 1, 445481.Google Scholar
Prelas, M.A., Boody, F. P., Miley, G.H. & Kunze, J. F. (1988). Nuclear driven flashlamps. Laser Part. Beams 6, 2562.Google Scholar
Radtsig, A.A. & Smirnov, B.M. (1986). Parameters of Atoms and Atomic Ions. Moscow: Energoatomizdat (in Russian).Google Scholar
Sakasai, K., Kakuta, T., Yamagishi, H., Nakazawa, M., Yamanaka, N. & Iguchi, T. (1996). Experiments for optical neutron detection using nuclear pumped laser. IEEE Trans. Nucl. Sci. 43, 15491553.Google Scholar
Tanaka, Y., Yoshino, K. & Freeman, D.E. (1975). Emission spectra of heteronuclear diatomic rare gas positive ions. J. Chem. Phys. 62, 44844496.Google Scholar
Ulrich, A. (2012). Light emission from the particle beam induced plasma: An overview. Laser Part. Beams 30, 199205.Google Scholar
Ulrich, A., Adonin, A., Jacoby, J., Turtikov, V., Fernengel, D., Fertman, A., Golubev, A., Hoffmann, D.H.H., Hug, A., Krucken, R., Kulish, M., Menzel, J., Morozov, A., Ni, P., Nikolaev, D.N., Shilkin, N.S., Ternovoi, V.Ya., Udrea, S., Varentsov, D. & Wieser, J. (2006). Excimer laser pumped by an intense, high-energy heavy-ion beam. Phys. Rev. Lett. 97, 153901.Google Scholar
Wieser, J., Ulrich, A., Fedenev, A. & Salvermoser, M. (2000). New interpretation of the third rare gas excimer continua. Proc. SPIE 4071, 248254.CrossRefGoogle Scholar
Xu, J. & Setser, D.W. (1990). Deactivation rate constants and product branching in collisions of the Xe(6p) states with Kr and Ar. J. Chem. Phys. 92, 41914202.Google Scholar
Zdorovets, M., Ivanov, I., Koloberdin, M., Kozin, S., Alexandrenko, V., Sambaev, E., Kurakhmedov, A. & Ryskulov, A. (2014). Accelerator complex based on DC-60 cyclotron. Proc. 24th Russian Particle Accelerator Conf., pp. 287289. Obninsk: FEI.Google Scholar