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Combinatorial Materials Science: What's New Since Edison?

Published online by Cambridge University Press:  31 January 2011

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Abstract

Combinatorial methods are high-efficiency methods to create large composition “libraries” of materials, for example, continuous composition variations, and test those compositions systematically in parallel for specific properties of interest, in contrast to the time-consuming one-composition-at-a-time approach. These methods have captured the attention of the materials industry with the promise of providing new discoveries “faster, better, and cheaper.” However, in the academic community, combinatorial methods often meet with less enthusiasm, perhaps due to the perception of combinatorial methodology as an Edisonian approach to science. The facts are quite to the contrary. In addition to impressive successes arising from the application of combinatorial methods to materials discovery, results coming out of systematic high-throughput investigations of complex materials phenomena (which would be too time-consuming or expensive to undertake) provide data leading to improvement in theories and models of materials chemistry and physics. Indeed, combinatorial methods provide a new paradigm for advancing a central scientific goal—the fundamental understanding of structure–property relationships of materials behavior.

Type
Research Article
Copyright
Copyright © Materials Research Society 2002

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References

1.Phillips, J.C., Physics of High-Tc Superconductors (Academic Press, New York, 1989).Google Scholar
2.Xiang, X.-D., Sun, X.-D., Briceño, G., Lou, Y., Wang, K.-A., Chang, H., Wallace-Freedman, W.G., Chen, S.-W., and Schultz, P.G., Science 268 (1995) p. 1738.CrossRefGoogle Scholar
3.Xiang, X.-D., Annu. Rev. Mater. Sci. 29 (1999) p. 149.CrossRefGoogle Scholar
4.Kennedy, K., Stefansky, T., Davy, G., Zackay, V.F., and Parker, E.R., J. Appl. Phys. 36 (1965) p. 3808.CrossRefGoogle Scholar
5.Miller, N.C. and Shirn, G.A., Appl. Phys. Lett. 10 (1967) p. 86.CrossRefGoogle Scholar
6.Hanak, J.J., Gittleman, J.I., Pellicane, J.P., and Bozowski, S., Phys. Lett. 30A (1969) p. 201.CrossRefGoogle Scholar
7.Sawatzky, E. and Kay, E., IBM J. Res. Develop. (November 1969) p. 696.CrossRefGoogle Scholar
8.Hanak, J.J., J. Mater. Sci. 5 (1970) p. 964.CrossRefGoogle Scholar
9.Hartsough, L.D. and Hammond, R.H., Solid State Commun. 9 (1971) p. 885.CrossRefGoogle Scholar
10.Hammond, R.H., Ralls, K.M., Meyer, C.H. Jr, Snowden, D.P., Kelly, G.M., and Pereue, J.H. Jr, J. Appl. Phys. 43 (1972) p. 2407;CrossRefGoogle Scholar
Hammond, R.H., Jacobson, B.E., Geballe, T.H., Talvacchio, J., Salem, J.R., Pohl, H.C., and Braginski, A.I., IEEE Trans. Magn. 15 (1979) p. 619;CrossRefGoogle Scholar
Kuo, J. and Geballe, T.H., Phys. Rev. B 23 (1981) p. 3230.Google Scholar
11.Berlincourt, T. (private communication).Google Scholar
12.van Dover, R.B., Hessen, B., Werder, D., Chen, C.-H., and Felder, R.J., Chem. Mater. 5 (1993) p. 32.CrossRefGoogle Scholar
13.Yoo, Y.K., Duewer, F.W., Yang, H., Yi, D., Li, J.-W., and Xiang, X.-D., Nature 406 (2000) p. 704.CrossRefGoogle Scholar
14.Oliver, W.C. and Pharr, G.M., J. Mater. Res. 7 (1992) p. 1564.CrossRefGoogle Scholar
15.Doerner, M.F. and Nix, W.D., J. Mater. Res. 1 (1986) p. 601.CrossRefGoogle Scholar
16.Zhao, J.-C., Adv. Eng. Mater. 3 (2001) p. 143.3.0.CO;2-F>CrossRefGoogle Scholar
17.Zhao, J.-C., J. Mater. Res. 16 (2001) p. 1565.CrossRefGoogle Scholar
18.Meredith, J.C., Karim, A., and Amis, E.J., Macromolecules 33 (2000) p. 5760.CrossRefGoogle Scholar
19.Meredith, J.C., Smith, A.P., Karim, A., and Amis, E.J., Macromolecules 33 (2000) p. 9747.CrossRefGoogle Scholar
20.Smith, A.P., Douglas, J., Meredith, J.C., Karim, A., and Amis, E.J., Phys. Rev. Lett. 87 (2001) p. 15503.CrossRefGoogle Scholar
21.Meredith, J.C., Karim, A., and Amis, E.J., in ACS Symposium Series: Combinatorial Approaches to Materials Development, edited by Malhotra, R. (American Chemical Society, Washington, DC, 2001).Google Scholar
22. For example, see High-Throughput Synthesis, edited by I. Sucholeiki (Marcel Dekker, New York, 2001).Google Scholar