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In situ and operando probing of solid–solid interfaces in electrochemical devices

Published online by Cambridge University Press:  10 October 2018

T.A. Wynn ,
J.Z. Lee ,
A. Banerjee  and
Y.S. Meng
T.A. Wynn
Affiliation:
University of California, San Diego, USA; twynn@eng.ucsd.edu
J.Z. Lee
Affiliation:
University of California, San Diego, USA; jzlee@eng.ucsd.edu
A. Banerjee
Affiliation:
University of California, San Diego, USA; a7banerjee@eng.ucsd.edu
Y.S. Meng
Affiliation:
University of California, San Diego, USA; shirleymeng@ucsd.edu
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Abstract

Solid-state electrolytes can offer improved lithium-ion battery safety while potentially increasing the energy density by enabling alkali metal anodes. There have been significant research efforts to improve the ionic conductivity of solid-state electrolytes and the electrochemical performance of all-solid-state batteries; however, the root causes of their poor performance—interfacial reaction and subsequent impedance growth—are poorly understood. This is due to the dearth of effective characterization techniques for probing these buried interfaces. In situ and operando methodologies are currently under development for solid-state interfaces, and they offer the potential to describe the dynamic interfacial processes that serve as performance bottlenecks. This article highlights state-of-the-art solid–solid interface probing methodologies, describes practical limitations, and describes a future for dynamic interfacial characterization.

Keywords

energy storageLiionic conductorphase equilibria
Type
Frontiers of Solid-State Batteries
Information
MRS Bulletin , Volume 43 , Issue 10: Frontiers of Solid-State Batteries , October 2018 , pp. 768 - 774
Copyright
Copyright © Materials Research Society 2018 

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