Hostname: page-component-cd9895bd7-gbm5v Total loading time: 0 Render date: 2024-12-28T19:46:23.263Z Has data issue: false hasContentIssue false

Evolution of Static Physical Properties in Plutonium by Self-irradiation Damage

Published online by Cambridge University Press:  01 February 2011

Brandon W Chung
Affiliation:
chung7@llnl.gov, Lawrence Livermore National Laboratory, Livermore, California, United States
Kenneth Lema
Affiliation:
lema1@llnl.gov, Lawrence Livermore National Laboratory, Livermore, California, United States
David Hiromoto
Affiliation:
hiromoto1@llnl.gov, Lawrence Livermore National Laboratory, Livermore, California, United States
Get access

Abstract

The alpha-decay of plutonium leads to the age-related change in physical properties. This paper presents updated results of age-related effects on enriched and reference alloys measured from immersion density, dilatometry, and mechanical tests. After nearly 100 equivalent years of aging, both the immersion density and dilatometry show that the enriched alloys are decreasing in density by less than 0.002% per year and now exhibit a near linear density decrease, without void swelling. The tensile tests show that the aging process increases the strength of plutonium alloys, followed by possible saturation past 70 equivalent years of age. The ultimate goal of this work is to develop capabilities to predict physical properties changed by aging effects.

Type
Research Article
Copyright
Copyright © Materials Research Society 2010

Access options

Get access to the full version of this content by using one of the access options below. (Log in options will check for institutional or personal access. Content may require purchase if you do not have access.)

References

1 Wolfer, W. G., “Radiation effects in plutonium. What is known? Where should we go from here,” in Los Alamos Science, eds. Cooper, N. G., (Los Alamos National Laboratory: Los Alamos, 2000, v26) pp 274285.Google Scholar
2 Hecker, S. S. and Martz, J. C., “Aging of Plutonium and its alloys,” in Los Alamos Science, eds. Cooper, N. G., (Los Alamos National Laboratory: Los Alamos, 2000, v26) pp 238243.Google Scholar
3 Chung, B. W., Thompson, S. R., Woods, C. H., Hopkins, D. J., Gourdin, W. H., and Ebbinghaus, B. B., J. Nucl. Mater., 335 142149 (2006).Google Scholar
4 Bowen, H. A. and Schoonover, R. M., J. of Res. Nat. Bur. Stand. – C, 71C [3] 179198 (1967).Google Scholar