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Holocene Precipitation Records from Inner Mongolia Derived from Hydrogen Isotope Compositions of Sediment Fatty Acids

Published online by Cambridge University Press:  25 September 2018

Qingmin Chen
Affiliation:
Shaanxi Center of Geological Survey, Shaanxi Institute of Geological Survey, Xi’an 710068, China
Weijian Zhou*
Affiliation:
State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an 710061, China
Zhe Wang
Affiliation:
Shaanxi Center of Geological Survey, Shaanxi Institute of Geological Survey, Xi’an 710068, China
Feng Xian
Affiliation:
State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an 710061, China
George S Burr
Affiliation:
State Key Laboratory of Loess and Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences, Xi’an 710061, China
*
*Corresponding author. Email: weijian@loess.llqg.ac.cn.

Abstract

The Inner Mongolian Plateau lies along the northern limit reached by the East Asian summer monsoon. This geographic setting makes it especially sensitive to environmental change and an excellent site for understanding Quaternary East Asian monsoon variability. In this study we present new results of hydrogen isotopic compositions of fatty acids extracted from sediments, which were used to construct Holocene paleoprecipitation (or moisture) changes in Northern China. The hydrogen isotopic composition (D/H ratio) of n-acids in the sedimentary sequence of the Duoerji peat, Inner Mongolia, was determined with gas chromatography and mass spectrometry. Changes in the precipitation from middle Inner Mongolia are recorded by the D/H ratio of n-C20, n-C22, n-C24, n-C26, n-C28 acids (δD). From 10–9 ka, the relatively high δD values indicate reduced precipitation in the Early Holocene. Subsequently, increased precipitation is reflected by reduced δD values from 9–5.5 ka. After 5.5 ka, gradually increasing δD values record an overall decrease in precipitation. The precipitation trends established for the Duoerji sequence are consistent with other major paleoclimate proxies in the East Asian monsoon region, especially with a distinct Holocene optimum of increased monsoonal activity from 9–5.5 ka. The δD resulting paleo-precipitation record clearly shows that the Holocene climate in Northern China is basically controlled by the insolation changes.

Type
Research Article
Copyright
© 2018 by the Arizona Board of Regents on behalf of the University of Arizona 

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References

REFERENCES

An, ZS. 2000. The history and variability of the East Asian paleomonsoon climate. Quaternary Science Reviews 19(1-5):171187.Google Scholar
An, ZS, Porter, SC, Kutzbach, JE, Wu, XH, Wang, SM, Liu, XD, Li, XQ, Zhou, WJ. 2000. Asynchronous Holocene optimum of the East Asian monsoon. Quaternary Science Review 19:743762.Google Scholar
Araguás-Araguás, L, Froehlich, K, Rozanski, K. 2000. Deuterium and oxygen-18 isotope composition of precipitation and atmospheric moisture. Hydrological Processes 14:13411355.Google Scholar
Battisti, DS, Ding, Q, Roe, GH. 2015. Coherent pan‐Asian climatic and isotopic response to orbital forcing of tropical insolation. Journal of Geophysical Research Atmospheres 119(21):11,997112,020.Google Scholar
Bowen, GJ. 2008. Spatial analysis of the intra-annual variation of precipitation isotope ratios and its climatological corollaries. Journal of Geophysical Research 113:D05113.Google Scholar
Brassell, SC, Eglinton, G, Marlowe, IT, Pflaumann, U, Sarnthein, M. 1986. Molecular stratigraphy: a new tool for climatic assessment. Nature 320:129133.Google Scholar
Bray, EE, Evans, ED. 1961. Distribution of n-paraffins as a clue to the recognition of source beds. Geochimica et Cosmochimica Acta 22:215.Google Scholar
Chen, CTA, Lan, HC, Lou, JY, Chen, YC. 2003. The dry Holocene megathermal in Inner Mongolia. Palaeogeography, Palaeoclimatology, Palaeoecology 19:181200.Google Scholar
Chen, FH, Yu, ZC, Yang, ML, Emi, I, Wang, S, David, BM, Huang, XZ, Yan, Z, Tomonori, SH, John, BB, Ian, B, Chen, JH, An, CB, Bernd, W. 2008. Holocene moisture evolution in arid central Asia and its out-of-phase relationship with Asian monsoon history. Quaternary Science Reviews 27(3–4):351364.Google Scholar
Clemens, SC, Prell, WL, Sun, YB. 2010. Orbital-scale timing and mechanisms driving late Pleistocene Indo-Asian summer monsoons: reinterpreting cave speleothem δ18O. Paleoceanography 25:545558.Google Scholar
Craig, H. 1961. Isotopic variations in meteoric waters. Science 133:17021703.Google Scholar
Cranwell, PA. 1974. Monocarboxylic acids in lake sediments: Indicators, derived from terrestrial and aquatic biota, of paleoenvironmental trophic levels. Chemical Geology 14:114.Google Scholar
Cranwell, PA. 1973. Chain-length distribution of n-alkanes from lake sediments in relation to post-glacial environmental change. Freshwater Biology 3:259265.Google Scholar
Dansgaard, W. 1964. Stable isotopes in precipitation. Tellus 16:436468.Google Scholar
Dayem, KE, Molnar, P, Battisti, DS, Roe, GH. 2010. Lessons learned from oxygen isotopes in modern precipitation applied to interpretation of speleothem records of paleoclimate from eastern Asia. Earth & Planetary Science Letters 295(1–2):219230.Google Scholar
Dykoski, CA, Edward, RL, Cheng, H, Yuan, DX, Cai, YJ, Zhang, ML, Lin, YS, Qing, JM, An, ZS, Revenaugh, J. 2005. A high-resolution, absolute-dated Holocene and deglacial Asian monsoon record from Donge Cave. China Earth Planetary Science Letters 233:7186.Google Scholar
Eglinton, G, Hamilton, RJ. 1967. Leaf epicuticular waxes. Science 156:13221334.Google Scholar
Ficken, KJ, Street-Perrott, FA, Perrott, RA, Swain, DL, Olago, DO, Eglinton, G. 1998. Glacial/interglacial variations in carbon cycling revealed by molecular and isotope stratigraphy of Lake Nkunga, Mt. Kenya, East Africa. Organic Geochemistry 29:17011719.Google Scholar
Gat, JR. 1996. Oxygen and hydrogen isotopes in the hydrologic cycle. Annual Review of Earth and Planetary Sciences 24:225262.Google Scholar
Guan, YY, Wamg, Y, Yao, PY, Chi, ZQ, Zhao, ZL. 2010. Environmental evolution since the Holocene in the Haolaihure antient lake, Keshitengqi, Inner Mongolia, China. Geological Bulletin of China 29:891900.Google Scholar
Heegaard, E, Birks, HJB, Telford, RJ. 2005. Relationships between calibrated ages and depth in stratigraphical sequences: an estimation procedure by mixed-effect regression. The Holocene 15:612618.Google Scholar
Hoffmann, G, Heimann, M. 1997. Water isotope modeling in the Asian monsoon region. Quaternary International 37:115128.Google Scholar
Hilkert AW, Douthitt CB, Schlüter HJ, Brand WA. 1999. Isotope ratio monitoring gas chromatography/mass spectrometry of D/H by high temperature conversion isotope ratio massspectrometry. Rapid Communications in Mass Spectrometry 13(13): 226–1230.Google Scholar
Hou, JZ, D’Andrea, WJ, Huang, YS. 2008. Can sedimentary leaf waxes record D/H ratios of continental precipitation? Field, model, and experimental assessments. Geochimica et Cosmochimica Acta 72:35033517.Google Scholar
Hou, JZ, D’Andrea, WJ, MacDonald, D, Huang, YS. 2007. Hydrogen isotopic variability in leaf waxes among terrestrial and aquatic plants around Blood Pond, Massachusetts (USA). Organic Geochemistry 38:977984.Google Scholar
Huang, YS, Shuman, B, Wang, Y, Webb, T. 2004. Hydrogen isotope ratios of individual lipids in lake sediments as novel tracers of climatic and environmental change: a surface sediment test. Journal of Paleolimnology 31:363375.Google Scholar
Ishiwatari, R, Hirakawa, Y, Uzaki, M, Yamada, K, Yada, T. 1994. Organic geochemistry of the Japan Sea sediments 1: bulk organic matter and hydrocarbon analyses of Core KH-79-3, C-3 from the Oki Ridge for paleoenvironment assessments. Journal of Oceanography 50:179195.Google Scholar
Jiang, YJ, Wang, W, Ma, YZ, Li, YY, Liu, LN, He, J. 2014. A preliminary study on Holocene climate change of Ordos plateau, as inferred by sedimentary record from Bojianghaizi lake of Inner Mongolia, China. Quaternary Sciences 34:654665.Google Scholar
Jin, HL, Su, ZZ, Sun, LY, Zhang, H, Jin, L. 2004. Holocene climatic change in Hunshandake desert. Chinese Science Bulletin 49:17301735.Google Scholar
Johnson, KR, Ingram, BL. 2004. Spatial and temporal variability in the stable isotope systematics of modern precipitation in China: Implications for paleoclimate reconstructions. Earth & Planetary Science Letters 220:365377.Google Scholar
Kutzbach, JE, Street-Perrott, FA. 1985. Milankovich forcing of fluctuations in the level of tropical lakes from 18 to 0 kyr BP. Nature 317:130134.Google Scholar
Liu, HY, Cui, HT, Tian, YH, Xu, LH. 2002. Temporal-Spatial variances of Holocene precipitation at the marginal area of the East Asian Monsoon influences from pollen evidence. Acta Botanica Sinica 44:864871.Google Scholar
Liu, JR, Song, XF, Yuan, GF, Sun, XM, Liu, X, Wang, SQ. 2010. Characteristics of δ18O in precipitation over Eastern Monsoon China and the water vapor sources. Chinese Science Bulletin 55:200211.Google Scholar
Liu, WG, Yang, H, Li, LW. 2006. Hydrogen isotopic compositions of n-alkanes from terrestrial plants correlate with their ecological life forms. Oecologia 150(2):330338.Google Scholar
Liu, WG, Yang, H. 2008. Multiple controls for the variability of hydrogen isotopic compositions in higher plant n-alkanes from modern ecosystems. Global Change Biology 14:21662177.Google Scholar
Liu, ZY, Wen, XY, Brady, EC, Otto-Bliesner, B, Yu, G, Lu, HY, Cheng, H, Wang, YJ, Zheng, WP, Ding, YH, Edwards, RL, Cheng, J, Liu, W, Yang, Hao. 2014. Chinese cave records and the East Asia summer monsoon. Quaternary Science Reviews 83:115128.Google Scholar
Logan, GA, Smiley, CJ, Eglinton, G. 1995. Preservation of fossil leaf waxes in association with their source tissues, Clarkia, northern Idaho, USA. Geochimica et Cosmochimica Acta 59(4):751763.Google Scholar
Meyers PA, Ishiwatari R. 1993. The Early Diagenesis of Organic Matter in Lacustrine Sediments. In: Engel MH, Macko SA, editors. Organic Geochemistry. New York: Plenum Press.Google Scholar
Mügler, I, Sachse, D, Werner, M, Xu, BQ, Wu, GJ, Yao, TD, Gleixner, G. 2008. Effect of lake evaporation on δD values of Nam Co (Tibetan Plateau) and Holzmaar (Germany). Organic Geochemistry 39:711729.Google Scholar
Nelson, DM, Henderson, AK, Huang, YS, Hu, FS. 2013. Influence of terrestrial vegetation on leaf wax δD of Holocene lake sediments. Organic Geochemistry 56:106110.Google Scholar
Nichols, J, Booth, RK, Jackson, ST, Pendall, EG, Huang, YS. 2011. Differential hydrogen isotopic ratios of sphagnum and vascular plant biomarkers in ombrotrophic peatlands as a quantitative proxy for precipitation-evaporation balance. Geochimica et Cosmochimica Acta 74:14071416.Google Scholar
Peng, YJ, Xiao, JL, Nakamura, T, Liu, BL, Inouchi, Y. 2005. Holocene East Asian monsoonal precipitation pattern revealed by grain-size distribution of core sediments of Daihai Lake in inner Mongolia of north-central China. Earth & Planetary Science Letters 233:467479.Google Scholar
Rao, ZG, Jia, GD, Qiang, MR, Zhao, Yan. 2014. Assessment of the difference between mid- and long chain compound specific δD n-alkanes values in lacustrine sediments as a paleoclimatic indicator. Original Research Article Organic Geochemistry 76:104117.Google Scholar
Ruddiman, WF. 2008. Earth’s Climate, Past and Future. 3rd edition. New York: Freeman and Company. p 117.Google Scholar
Sachse, D, Radke, J, Gleixner, G. 2004. Hydrogen isotope ratios of recent lacustrine sedimentary n-alkanes record modern climate variability. Geochimica et Cosmochimica Acta 68:48774889.Google Scholar
Seki, O, Meyers, PA, Kawamura, K, Zheng, YH, Zhou, WJ. 2009. Hydrogen isotopic ratios of plant wax n-alkanes in a peat bog deposited in northeast China during the last 16 kyr. Organic Geochemistry 40:671677.Google Scholar
Sessions, AL, Burgoyne, TW, Schimmelmann, A, Hayes, JM. 1999. Fractionation of hydrogen isotopes in lipid biosynthesis. Organic Geochemistry 30(9):11931200.Google Scholar
Shi, YF, Kong, ZC, Wang, SM, Tang, LY, Wang, FB, Yao, TD, Zhao, XT, Zhang, PY, Shi, SH. 1992. Climate fluctuations and important events of Holocene Megathermal in China. Science in China Series B 12:13001307.Google Scholar
Sternberg, L, da, SL. 1988. D/H ratios of environmental water recorded by D/H ratios of plant lipids. Nature 333:5961.Google Scholar
Sun, QL, Wang, SM, Zhou, J, Shen, J, Cheng, P, Xie, XP, Wu, F. 2009. Lake surface fluctuations since the late glaciation at Lake Daihai, North central China: A direct indicator of hydrological process response to East Asian monsoon climate. Quaternary International 194:4554.Google Scholar
Sun, QL. 2005. Climate and environment evolution since the last Deglaciation recorded by the lacustrine sediments from Lake Daihai [PhD dissertation]. Graduate School of the Chinese Academy of Science (Institute of Earth Environment). In Chinese.Google Scholar
Wang, FY, Sun, XJ. 1997. A preliminary study on paleoenvironmental evolution during the Holocene from Chasuqi peat profile in Inner Mongolia. Chinese Science Bullelin 42:514518. In Chinese.Google Scholar
Wang, HY, Liu, HY, Zhao, FJ, Yin, Y, Zhu, JL, Ian, S. 2012. Early- and mid-Holocene palaeoenvironments as revealed by mineral magnetic, geochemical and palynological data of sediments from Bai Nuur and Ulan Nuur, southeastern inner Mongolia Plateau, China. Quaternary International 250:100118.Google Scholar
Wang, YJ, Cheng, H, Edwards, RL, He, YQ, Kong, XG, An, ZS, Wu, JY, Kelly, MJ, Dykoski, CA, Li, XD. 2005. The Holocene Asian Monsoon: links to solar changes and North Atlantic climate. Science 308:854857.Google Scholar
Wen, RL, Xiao, JL, Chang, ZG, Zhai, DY, X, QH, Li, YC. 2010. Holocene climate changes in the mid-high-latitude-monsoon margin reflected by the pollen record from Hulun Lake, northeastern inner Mongolia. Quaternary Research 73:293303.Google Scholar
Wiesenberg, GLB, Schwark, L. 2006. Carboxylic acid distribution patterns of temperate C3, and C4 crops. Organic Geochemistry 37(12):19731982.Google Scholar
Xiao, JL, Xu, QH, Nakamura, T, Yang, XL, Liang, WD, Inouchi, Y. 2004. Holocene vegetation variation in the Daihai Lake region of north-central China: a direct indication of the Asian monsoon climatic history. Quaternary Science Reviews 2:16691679.Google Scholar
Xu, W, Cui, LL, Xiao, JL, Ding, ZL. 2013. Stable carbon isotope of black carbon in lake sediments as an indicator of terrestrial environmental changes: An evaluation on paleorecord from Daihai Lake, Inner Mongolia, China. Chemical Geology 347:123134.Google Scholar
Yang, H, Huang, YS. 2003. Preservation of lipid hydrogen isotope ratios in Miocene lacustrine sediments and plant fossils at Clarkia, northern Idaho, USA. Organic Geochemistry 34:413423.Google Scholar
Yao, Y, Yang, H, Liu, WG, Li, XZ, Chen, YW. 2015. Hydrological changes of the past 1400 years recorded in D of sedimentary n-alkanes from Poyang Lake, southeastern China. Holocene 518(3):9499.Google Scholar
Yin, Y, Liu, HY, He, SY, Zhao, FJ, Zhu, JL, Wang, HY, Liu, G, Wu, XC. 2011. Patterns of local and regional grain size distribution and their application to Holocene climate reconstruction in semi-arid Inner Mongolia, China. Palaeogeography, Palaeoclimatology, Palaeoecology 307:168176.Google Scholar
Yun, H. 1987. Country Annals of Turmot. Inner Mongolia Peoples Publishing House. In Chinese.Google Scholar
Zhai, DY, Xiao, JL, Zhou, L, Wen, RL, Chang, ZG, Wang, X, Jin, XD, Pang, QQ, Shigeru, I. 2011. Holocene East Asian monsoon variation inferred from species assemblage and shell chemistry of the ostracodes from Hulun Lake, Inner Mongolia. Quaternary Research 7:512522.Google Scholar
Zhou, WJ, An, ZS, Lin, BH, Xiao, JL, Zhang, JZ, Xie, J, Zhou, MF. 1992. Chronology of the Baxie loess profile and the history of monsoon climates in China between 17,000 and 6000 years BP. Radiocarbon 34:818825.Google Scholar
Zhou, WJ, Lu, XF, Wu, ZK, Deng, L, Jull, AJT, Donahue, D, Beck, JW. 2002. Peat record reflecting Holocene climatic change in the Zoige Plateau and AMS radiocarbon dating. Chinese Science Bulletin 47:6670.Google Scholar
Zhou, WJ, Yu, XF, Jull, AJT, Burr, G, Xiao, JY, Lu, XF. 2004. High-resolution evidence from southern china of an Early Holocene optimum and a mid-Holocene dry event during the past 18,000 years. Quaternary Research 62:3948.Google Scholar
Zhou, WJ, Zheng, YH, Meyers, PA, Jull, AJT, Xie, SC. 2010. Postglacial climate-change record in biomarker lipid compositions of the Hani peat sequence, Northeastern China. Earth & Planetary Science Letters 294:3746.Google Scholar