We demonstrate efficient and economical all-solid-state post-compression based on dual-stage periodically placed thin fused silica plates driven by a more than 100 W ytterbium-doped yttrium aluminum garnet Innoslab amplifier seeded by a fiber frontend. Not only is a more than eight-fold pulse compression with 94% transmission achieved, but also the pulse quality and spatial mode are improved, which can be attributed to the compensation for the residual high-order dispersion and the spatial mode self-cleaning effect during the nonlinear process. It enables a high-power ultrafast laser source with 64 fs pulse duration, 96 W average power at 175 kHz repetition rates and good spatiotemporal quality. These results highlight that this all-solid-state post-compression can overcome the bandwidth limitation of Yb-based lasers with exceptional efficiency and mitigate the spatiotemporal degradation originating from the Innoslab amplifier and fiber frontend, which provides an efficient and economical complement for the Innoslab laser system and facilitates this robust and compact combination as a promising scheme for high-quality higher-power few-cycle laser generation.

A novel method, combining an asymmetric four-grating compressor (AFGC) with pulse post-compression, is numerically demonstrated to improve the spatial uniformity of laser beams and hence to suppress small-scale self-focusing (SSSF) during the beam propagation in nonlinear materials of high peak power lasers. The spatial uniformity of laser beams is an important factor in performing post-compression, due to the spatial intensity modulation, or hot spots will be aggravated during the nonlinear propagation and then seriously damage the subsequent optical components. Three-dimensional numerical simulations of post-compression are implemented based on a femtosecond laser with a standard compressor and an AFGC, respectively. The simulated results indicate that post-compression with the AFGC can efficiently suppress the SSSF and also shorten the laser pulses from 30 fs to sub-10 fs. This work can provide a promising route to overcome the challenge of SSSF and will be meaningful to promote the practical application of the post-compression technique in high peak power lasers.

We demonstrate the generation, spectral broadening and post-compression of second harmonic pulses using a thin beta barium borate (BBO) crystal on a fused-silica substrate as the nonlinear interaction medium. By combining second harmonic generation in the BBO crystal with self-phase modulation in the fused-silica substrate, we efficiently generate millijoule-level broadband violet pulses from a single optical component. The second harmonic spectrum covers a range from long wave ultraviolet (down to 310 nm) to visible (up to 550 nm) with a bandwidth of 65 nm. Subsequently, we compress the second harmonic beam to a duration of 4.8 fs with a pulse energy of 0.64 mJ (5 fs with a pulse energy of 1.05 mJ) using chirped mirrors. The all-solid free-space apparatus is compact, robust and pulse energy scalable, making it highly advantageous for generating intense second harmonic pulses from near-infrared femtosecond lasers in the sub-5 fs regime.

The post-compression technique based on self-phase modulation of high-energy pulses leads to an increase in achievable peak power and intensity. Typically, the pulses considered in experiments have been less than 100 fs in duration. Here, the method is applied to the ELFIE laser system at the LULI facility, for a pulse of 7 J energy and an initial measured duration of 350 fs. A 5-mm-thick fused silica window and a 2 mm cyclic-olefin polymer were used as optical nonlinear materials. The 9 cm diameter beam was spectrally broadened to a bandwidth corresponding to 124 fs Fourier-limited pulse duration, and then it was partly post-compressed to 200 fs. After measuring the spatial spectra of the beam fluence, a uniform gain factor of 4 increase in the fluctuations over the studied range of frequencies is observed, due to small-scale self-focusing.

We demonstrate an efficient ultrafast source with 195 fs pulse duration, 54 W average power at 200 kHz repetition rate and near diffraction-limited beam quality. The compact setup incorporates a thin-disk Yb:YAG regenerative amplifier (RA) and a subsequent nonlinear pulse compression stage with periodic-layered Kerr media (PLKM), which is one of the multiple-thin-solid-plate schemes based on nonlinear resonator theory. In virtue of the formation of quasi-stationary spatial soliton in PLKM, the near diffraction-limited beam quality of the RA remained almost undisturbed after post-compression. The nonlinear pulse compression module is simple and efficient with a transmission of 96%. To the best our knowledge, for pulse energy over 200 μJ, this is the highest output power reported for the multiple-thin-solid-plate scheme. This source manifests an economical combination to mitigate the bandwidth limitations of Yb-based high-power chirped pulse amplifiers.

Spectral-broadening of the APOLLON PW-class laser pulses using a thin-film compression technique within the long-focal-area interaction chamber of the APOLLON laser facility is reported, demonstrating the delivery of the full energy pulse to the target interaction area. The laser pulse at 7 J passing through large aperture, thin glass wafers is spectrally broadened to a bandwidth that is compatible with a 15-fs pulse, indicating also the possibility to achieve sub-10-fs pulses using 14 J. Placing the post-compressor near the interaction makes for an economical method to produce the shortest pulses by limiting the need for high damage, broadband optics close to the final target rather than throughout the entire laser transport system.

We report on compact and robust supercontinuum generation and post-compression using transmission of light through multiple thin solid plates at the SwissFEL X-ray free-electron laser facility. A single stage consisting of three thin plates followed by a chirped mirror compressor achieves compression of initially 30-fs pulses with 800-nm center wavelength to sub-10-fs duration. We also demonstrate a two-stage implementation to compress the pulses further to sub-5-fs duration. With the two-stage setup, the generated supercontinuum includes wavelengths ranging from 500 to 1100 nm. The multi-plate setup is compact, robust, and stable, which makes it ideal for applications at free-electron laser facilities such as pump-probe experiments and laser-arrival timing tools.

The input pulse of the laser PEARL with energy of 18 J and pulse duration of about 60 fs was compressed to 10 fs after passage through a 4-mm-thick KDP crystal and reflection at two chirped mirrors with sum dispersion of −200 fs2. The experiments were performed for the В-integral values from 5 to 19 without visible damage to the optical elements, which indicates that small-scale self-focusing is not a significant issue. It was shown that, by virtue of the low dispersion of the group velocity, the KDP crystal has some advantages over silica: a larger pulse compression coefficient, especially at a small value of the В-integral (B = 5, …, 9), lower absolute values of chirped mirror dispersion, and also a possibility to control the magnitude of nonlinearity and dispersion by changing crystal orientation.