Swelling soils, particularly those rich in smectite, present significant challenges to civil engineering due to their shrinking–swelling behaviour. Lime stabilization is a commonly used practice to address this, but the reactivity of smectite minerals in an alkaline limestone environment differs widely. This study investigates the reactivity of two Moroccan smectite-rich clays – montmorillonite-dominated bentonite and stevensite/saponite-rich bentonite – when treated with aerial lime. Through mineralogical, microstructural and mechanical analyses, this study highlights the distinct behaviour of montmorillonite, which reacts with lime to form calcium silicate hydrate gels, compared to the inert response of stevensite/saponite. Despite its low pozzolanic activity, stevensite-bentonite demonstrates greater mechanical strength, reaching 2.5 MPa in the S3 mixture (90% stevensite-bentonite and 10% lime). This strength is attributed to the formation of calcite through the de-dolomitization of dolomite. The findings reveal different stabilization mechanisms between dioctahedral and trioctahedral smectites, offering new insights for soil stabilization strategies involving these smectite types.