Laser pulses are largely used for processing and analysis of materials and in particular for nano-particle synthesis. This paper addresses fundamentals of the generation of nano-materials following specific thermodynamic paths of the irradiated material. Computer simulations using the hydro code MULTI and the SESAME equation of state have been performed to follow the dynamics of a target initially heated by a short laser pulse over a distance comparable to the metal skin depth.

A theoretical model of soft X-ray emission from laser irradiated clusters is developed. An intense short pulse laser of Gaussian radial and temporal profiles impinged on a clustered gas jet, heats the cluster electrons, leading to Bremsstrahlung emission of X-rays. As the clusters expand under hydrodynamic pressure, plasma frequency of the cluster electrons ωpe decreases. When plasma frequency of a cluster approaches plasma resonance ${\rm \omega}_{\,pe} = \sqrt{3} {\rm \omega}$ (where ω is the laser frequency), the electrons are resonantly heated by the laser and a rapid rise in X-ray emission occurs. After a while, when cluster expansion detunes the plasma resonance, X-ray emission falls off.

A space-resolved charge density of ions is derived from a time-resolved current of ions emitted from laser-produced plasma and expanded into the vacuum along collision-free and field-free paths. This derivation is based on a similarity relationship for ion currents with “frozen” charges observed at different distances from the target. This relationship makes it possible to determine a map of ion charge density at selected times after the laser plasma interaction from signals of time-of-flight detectors positioned at a certain distance from the target around a target-surface normal. In this work, we present maps of the charge density of ions emitted from Cu and polyethylene plasmas. The mapping demonstrates that bursts of ions are emitted at various ejection angles ϕn with respect to the target-surface normal. There are two basic directions ϕ1 and ϕ2, one belonging to the fastest ions, i.e., protons and carbon ions, and the other one to the slowest ions being a part of each plasma plume.

A formalism for investigation of the propagation characteristics of various order short duration (pico second) Gaussian/dark hollow Gaussian laser pulse (DHGP) in a tunnel ionized plasma has been developed, which takes into account the electron-ion recombination. Utilizing the paraxial like approach, a nonlinear Schrödinger wave equation characterizing the beam spot size in space and time has been derived and solved numerically to investigate the transverse focusing (in space) and longitudinal compression (in time) of the laser pulse; the associated energy localization as the pulse advances in the plasma has also been analyzed. It is seen that in the absence of recombination the DHGP and Gaussian pulse undergo oscillatory and steady defocusing respectively. With the inclusion of recombination, the DHGP and Gaussian pulse both undergo periodic self-focusing for specific parameters. The DHGPs promise to be suitable for enhancement of energy transport inside the plasma.

Non-equilibrium heat transfer described by a two-step temperature model was developed to study the thermal evolution through target materials irradiated by femtosecond laser pulse. Two-dimensional heat transfer equations were solved numerically. The temperature dependent thermo-physical properties of the electron and the lattice are considered in the model. The Gaussian spatial and temporal distribution of the heat and temperature of the electron and the lattice is presented. The effect of reflectivity, electron — lattice coupling factor, and the spot size was studied using copper targets.

Thermonuclear ignition and burn propagation in pre-compressed cylindrical deuterium-tritium (DT) targets is studied by two-dimensional radiation hydrodynamics simulations using the code MULTI-2D. Special attention is paid to self-sustained steady burn wave propagation. Peak temperatures and burn wave velocity scale with the density-radius product of the fuel, and wave propagation is obtained for (ρR)DT ≥ 0.45 g/cm2. Radiation transport is identified as the dominant mechanism to drive the wave. Details of ignition by a heavy ion beam pulse are also presented. Limitations in the physics basis of the simulations are pointed out. The results are compared with previous publications found in the literature.

Laser surface melting is one of the most important processes in laser material processing. Selective vaporization of alloying elements in laser melting offers fundamental understanding of laser processing on metallic alloys. This work provides linkage between laser melting and material properties using secondary ion mass spectrometry (SIMS) for tiny vaporized species in laser-generated plume and energy dispersive spectroscopy (EDS) for solid solution range in molten pool, both qualitatively and quantitatively (up to hundreds of micron). Silicon wafer was used to collect the generated plume. Chemical analysis was carried out on top surface and sub-surface of the deposited plume. Transport behavior as well as distribution of the vaporized species inside the plume was further proposed.

We report utilization of the laser induced forward transfer technique to re-deposit indium thin films onto the accepter substrate using nJ laser pulses from a femtosecond laser oscillator. Keeping the accepter substrate stationary enables dots of Indium to be deposited; in contrast, linear motion of the accepter substrate facilitates deposition of lines of Indium. The effect of laser pulse energy on the deposition process is studied. The effect of translation speed of donor substrate on the laser induced forward transfer pattern is also probed and an upper limit of translation speed is established beyond which smearing is observed to occur.

One of the numerous applications of the ICAN laser using the advantage of fiber optics with chirped pulse amplification (CPA), is the scheme of side-on initiation of a nuclear fusion flame in solid density fuel with laser pulses of shorter than picosecond (ps) duration and power in the petawatt (PW) and higher range. The ICAN Fiber optics has special advantages with the potential that >900 PW spherical laser pulses may ignite the proton reaction with 11B (HB11) without the problem of dangerous radioactive radiation. Though secondary reactions can be estimated very roughly, the feasibility of a power station with the necessary energy gains can be concluded.

The remaining challenges, developing the relativistic electron beam sources, stimulate the investigations of cathode materials. Carbon-fiber-aluminum composite is the most appropriate cathode materials to construct the robust relativistic electron beam sources. Carbon-fiber-aluminum composite is treated by a non-equilibrium atmospheric plasma torch with a copper electrode based on high-voltage gas discharge. The axial and radial distributions of the plasma torch temperature are measured to determine the optimal treatment temperature and location. Copper-oxide particles with diameters of less than 1 µm are deposited onto the surface of the carbon-fibers and a layer of copper-oxide covers the entire surface as the treatment time is increased. Raman spectroscopy suggests that although the locations of the D and G band are similar, the areas of the D and G bands increase after the plasma treatment due to the reduced graphite crystalline size in the carbon-fibers. Analysis of the copper electrode surface discloses materials ablation arising from the discharge which releases copper from the source. Our results reveal that the atmospheric plasma torch generated by high-voltage discharge is promising in the surface modification of the carbon-fiber-reinforced aluminum composite. Further, the plasma produced by atmospheric plasma torch is dusty plasma, due to the participation of liberated copper particles. The plasma torch was analyzed by fluid dynamics, in terms of plasma density, plasma expansion velocity, and internal pressure, and it was found that the plasma produced by atmospheric torch is supersonic flow.

Collisional effects on the current-filamentation instability (CFI), accounting for the space charge effect (SCE), are investigated kinetically for a relativistic beam propagating in dense plasmas. It is shown that collisions can completely suppress the SCE in low temperature dense plasma, leading to enhancement of the CFI. This kind of decoupling mechanism is quite different from the well-known resistive mechanism [Molvig (1975). Phys. Rev. Lett. 35, 1504]. In particular, we find the present decoupling mechanism can well explain the recent numerical simulation results [Karmakar et al. (2008). Phys. Rev. Lett. doi: 101, 255001]. In the parameter regime related to the laser-solid interaction and fast ignition scenario (FIS), the CFI growth rate with SCE included is enhanced in the low plasma density region through the decoupling mechanism. In the high plasma density region, it is enhanced mainly through the resistive mechanism.

It is shown that in the focus of ultra-short pulses of duration t, the equivalent relation s = ct, where c is the speed of light and s the spatial extent of the pulse of the collimated pulse, does not hold. While the duration of one pulse is constant and independent of the measurement point, the spatial extension of the ultra-short pulse can be spatially shorter a factor more than 10 compared to the one obtained from the usual relation. The result is explained in correspondence with the extension of the Rayleigh range. Few femtosecond long gamma bursts can thus be generated in Thomson backscattering experiments performed in the lambda cube regime.

High-voltage pulse modulator has broad applications in industry. In order to pursue the qualities of compactness, solidification, and long life time, a high-voltage pulse modulator based on a helical Blumlein pulse forming line (HBPFL),a Marx generator and a self-coupling saturable pulse transformer (SPT) with fully cylindrical coaxial conductors is put forward and investigated in this paper. A new method that the fully cylindrical SPT simultaneously works as the charging pulse transformer and magnetic switch of the HBPFL is put forward and demonstrated. Traditional spark gap is substituted by the SPT to enable the features of solidification, compactness, and long life time of the modulator. Experimental results showed that the SPT had good response characteristics to short sinusoidal pulse and 100 ns-range square pulses. The fully cylindrical SPT driven by the 50–70 kV Marx generator can suppress the saturated inductance of the secondary windings to a level less than 500 nH, due to the strong reversed mutual induction between cylindrical windings after the core saturated. It also demonstrated that the pulse modulator was able to deliver a high-voltage pulse to a 160 Ω load, with amplitude of 148 kV, pulse duration of 130 ns, and pulse rise time ranging from 60 to 105 ns.

For the purpose of material studies for future nuclear fusion reactors, the IFMIF deuteron beams present a simultaneous combination of unprecedentedly high intensity (2 × 125 mA CW), power (2 × 5 MW) and space charge. Special considerations and new concepts have been developed in order to overcome these challenges. The global strategy for beam dynamics design of the 40 MeV IFMIF accelerators is presented, stressing on the control of micro-losses, and the possibility of online fine tuning. Start-to-end simulations without and with errors are presented for the prototype accelerator. Considerations about conflicts between halo and emittance minimization are then discussed in this very high space charge context.

The effect of laser-irradiance on the surface morphology and laser induced breakdown spectroscopy of zinc has been investigated by employing Nd:YAG laser (wavelength λ = 1064 nm, pulse duration t ~ 10 ns, and repetition rate = 10 Hz) under ambient environment of argon at a pressure of 20 Torr. For this purpose, zinc targets were exposed to various laser irradiances ranging from 13 GW/cm2 to 100 GW/cm2. Scanning electron microscope analysis has been performed to analyze the surface modification of irradiated zinc targets. Scanning electron microscope analysis revealed the formation of various kinds of structures such as ripples, cones, cavities, and wave like ridges at the center and peripheral regions of ablated zinc. In the central ablated region with increasing laser irradiance, the growth of distinct and well defined ripples is observed. Further increase in irradiance makes the appearance of these ripples diffusive and narrow. In order to correlate the plasma parameters with the surface modification, laser induced breakdown spectroscopy analysis has also been performed. The electron temperature and number density of zinc plasma have been evaluated at various laser irradiances. For both plasma parameters, an increasing trend up to a certain value of laser irradiance is observed which is due to enhanced energy deposition. Afterword a decreasing trend is achieved which is attributed to the shielding effect. With further increase in irradiance a saturation stage comes and almost no change in plasma parameters is observed. This saturation is explainable on the basis of the formation of a self-regulating regime near the target surface. A strong correlation between surface modification and plasma parameters is established.

In this paper, a new method for efficient generation of high-energy ion bunches via laser-induced cavity pressure acceleration (LICPA) is examined using one-dimensional particle-in-cell code PIC1D. It is found that for high laser beam intensities of the order of 1022 W/cm2 and for circular light polarization, a substantial increase in parameters of the accelerated ions is obtained when the target is placed inside a special cavity, into which the laser beam is introduced by a small hole. As compared to the pure radiation pressure acceleration scheme, the LICPA scheme leads to an increase in ion energies and the laser-to-ions energy conversion efficiency while the width of the ion energy spectrum are similar for both the schemes. Such a tendency was observed for all carbon targets (from 2 µm to 0.2 µm thick) investigated in the paper. The results of PIC1D simulations agree very well with predictions of the suitably generalized light sail model.

In this work, we present the spectroscopic studies of the plasma generated at the surface of manganese sulfate by the fundamental (1064 nm) and second harmonic (532 nm) of a Q-switched Nd:YAG laser. The 4s4p 4F7/2→ 4s 2H9/2 at 438.80 nm, 4p 2I11/2 → 4s22I11/2 at 440.80 nm, 4p 4G11/2 → 4s 2H9/2 at 464.27 nm, 4p 4F5/2→ 4s 4D7/2 at 467.16, 4p 4F5/2 → 4s24G 7/2 at 515.08 nm, and 4p 4F7/2 → 4s2 4G 9/2 at 519.65 nm transitions have been used to estimate the electron temperature through the Boltzmann plot method. The number density has been estimated from the Stark broadened profiles of the spectral line 348.30 nm. The spatial behavior of the electron temperature and number density has been examined at different ambient air pressures and with laser irradiance. The temperature and number density are found to be in the range from 9842 K to 9371 K and 1.58 × 1017 to 3.26 × 1016 cm−3 for the 1064 nm laser, from 9668 to 9297 K and 2.27 × 1017 to 5.79 × 1016 cm−3 for the 532 nm laser.

Laser interactions with spray targets (clouds of submicron droplets) are studied here via numerical simulations using two-dimensional particle-in-cell codes. Our simulations demonstrate an efficient absorption of laser pulse energy inside the spray. The energy absorption efficiency depends on the inter-droplet distance, size of the cloud of droplets, and laser pulse intensity, as well as on the pre-evaporation of droplets due to laser pulse pedestal. We investigate in detail proton acceleration from the spray. Energy spectra of protons in various acceleration directions vary significantly depending on the density profile of the plasma created from the droplets and on laser intensity. The spray target can be alternative of foil targets for high intensity high repetition ultrahigh contrast femtosecond lasers. However, at intensities >1021 W/cm2, the efficiency of laser absorption and ion acceleration from the droplets drops significantly in contrast to foils.

The effects of a radiation field (RF) on the interaction process of a relativistic electron beam (REB) with an electron plasma are investigated. The stopping power of the test electron averaged with a period of the RF has been calculated assuming an underdense plasma, ω0 > ωp, where ω0 is the frequency of the RF and ωp is the plasma frequency. In order to highlight the effect of the radiation field we present a comparison of our analytical and numerical results obtained for nonzero RF with those for vanishing RF. In particular, it has been shown that the weak RF increases the mean energy loss for small angles between the velocity of the REB and the direction of polarization of the RF while decreasing it at large angles. Furthermore, the relative deviation of the energy loss from the field-free value is strongly reduced with increasing the beam energy. Special case of the parallel orientation of the polarization of the RF with respect to the beam velocity has been also considered. At high-intensities of the RF two extreme regimes have been distinguished when the excited harmonics cancel effectively each other reducing strongly the energy loss or increasing it due to the constructive interference. Moreover, it has been demonstrated that the energy loss of the ultrarelativistic electron beam increases systematically with the intensity of the RF exceeding essentially the field-free value.

One-dimensional particle-in-cell and Monte-Carlo (FLUKA) simulation methods were used together, in order to investigate the production of positrons in lead targets, illuminated by a short-pulse high-intensity laser. The study is focused on lead targets of 1 mm thickness and more and pulses of intensity in the range 1019–1022 W/cm2. The calculations provided an estimate of an absolute number of positrons and the ratio of electrons and positrons emerging from the target. The thickness of the target is scaled in order to find an optimal thickness that could provide a neutral electron-positron beam.