The International Conference on “Ultrashort High-Energy Radiation and Matter” has been held in Villa Monastero, Varenna, Italy, during October 7–10, 2003. The conference has been jointly organized by the “Piero Caldirola” International Centre for the Promotion of Science and International School of Plasma Physics, Milan, Italy, and by the FEMTO Programme of the European Science Foundation (chaired by Prof. Charles Joachain of the University of Bruxelles).

We present a Ramsey technique using high-order harmonics for high-resolution atomic spectroscopy in the extreme ultraviolet. Pairs of time-delayed and phase-coherent harmonic pulses generated by the interaction of ultrashort and intense laser pulses with a noble gas are used to study excited states of krypton.

At high laser intensities, three step recollision processes such as high order harmonic generation and high-order ATI, are normally severely suppressed due to the magnetic field component of the laser pulse. However, if the laser pulse and relativistic ion beam are directed against each other, a significant increase in the frequency and the intensity of the pulse in the rest frame of the ions can occur. By performing calculations based on a Coulomb-corrected nondipole strong field approximation, we have shown that there is a range of intensities, Lorentz factors, and ion charges for which the suppression of the three step recollision processes is not severe, even for ponderomotive energies exceeding 10 keV. As an example, we consider parameters relevant to the accelerator that will be built at GSI-Darmstadt, capable of accelerating multicharged ions to Lorentz factors reaching 30.

We report results from a study of the integrated column density and expansion dynamics of ground-state-selected Ba+ ions in a laser–plasma plume using a new experimental system—VPIF (vacuum-ultraviolet photoabsorption imaging facility). The ions are tracked by recording the attenuation of a pulsed and collimated vacuum ultraviolet beam, tuned to the 5p–6d inner-shell resonance of singly ionized barium, as the expanding plasma plume moves across it. The attenuated beam is allowed to fall on a CCD array where the spatial distribution of the absorption is recorded. Time-resolved ion velocity and integrated column density maps are readily extracted from the photoionization images.

High-resolution K-shell spectra of a plasma created by superintense laser irradiation of micron-sized Ar clusters have been measured with an intensity above 1019 W/cm2 and a pulse duration of 30 fs. The total photon flux of 2 × 108 photons/pulse was achieved for Heα1 resonant line of Ar (λ = 3.9491 Å, 3.14 keV). In parallel with X-ray measurements, energy distributions of emitted ions have been measured. The multiply charged ions with kinetic energies up to 800 keV were observed. It is found that hot electrons produced by high contrast laser pulses allow the isochoric heating of clusters and shift the ion balance toward the higher charge states, which enhances both the X-ray line yield of the He-like argon ion and the ion kinetic energy.

The Compton scattering of a terawatt-class, femtosecond laser pulse by a high-brightness, relativistic electron beam has been demonstrated as a viable approach toward compact, tunable sources of bright, femtosecond, hard X-ray flashes. The main focus of this article is a detailed description of such a novel X-ray source, namely the PLEIADES (Picosecond Laser–Electron Inter-Action for the Dynamical Evaluation of Structures) facility at Lawrence Livermore National Laboratory. PLEIADES has produced first light at 70 keV, thus enabling critical applications, such as advanced backlighting for the National Ignition Facility and in situ time-resolved studies of high-Z materials. To date, the electron beam has been focused down to σx = σy = 27 μm rms, at 57 MeV, with 266 pC of charge, a relative energy spread of 0.2%, a normalized horizontal emittance of 3.5 mm·mrad, a normalized vertical emittance of 11 mm·mrad, and a duration of 3 ps rms. The compressed laser pulse energy at focus is 480 mJ, the pulse duration 54 fs Intensity Full Width at Half-Maximum (IFWHM), and the 1/e2 radius 36 μm. Initial X rays produced by head-on collisions between the laser and electron beams at a repetition rate of 10 Hz were captured with a cooled CCD using a CsI scintillator; the peak photon energy was approximately 78 keV, and the observed angular distribution was found to agree very well with three-dimensional codes. The current X-ray dose is 3 × 106 photons per pulse, and the inferred peak brightness exceeds 1015 photons/(mm2 × mrad2 × s × 0.1% bandwidth). Spectral measurements using calibrated foils of variable thickness are consistent with theory. Measurements of the X-ray dose as a function of the delay between the laser and electron beams show a 24-ps full width at half maximum (FWHM) window, as predicted by theory, in contrast with a measured timing jitter of 1.2 ps, which contributes to the stability of the source. In addition, K-edge radiographs of a Ta foil obtained at different electron beam energies clearly demonstrate the γ2-tunability of the source and show very good agreement with the theoretical divergence-angle dependence of the X-ray spectrum. Finally, electron bunch shortening experiments using velocity compression have also been performed and durations as short as 300 fs rms have been observed using coherent transition radiation; the corresponding inferred peak X-ray flux approaches 1019 photons/s.

X-ray spectra of H-like Mg ions produced in a laser plasma have been measured by space-resolved high-resolution spectroscopy. We identified satellite lines near Lyα lines, 2lnl′ − 1snl′ + hν for n = 2, 3, and 4. We construct a collisional radiative model including the doubly excited states for the intensity ratios of satellite lines. We use atomic data calculated by different methods for satellite lines and compare the results. We derive the electron temperature and density of the laser-produced plasma by a new technique using intensity ratios of only satellite lines. This technique is useful because the Lyα lines are often affected by opacity.

Ray-tracing simulations of an optical X-ray system based on a spherically bent crystal operating in Bragg configuration for monochromatic projection imaging of thin samples are presented, obtained using a code developed for that purpose. The code is particularly suited for characterizing experimental arrangements routinely used with laser-produced plasma X-ray sources. In particular, the spatial resolution of the imaging system was investigated and a careful study of the complex pattern of the X-ray backlighting beam was performed.

Within the next few years X-ray free-electron lasers (XFELs) now under construction are expected to generate highly collimated XUV pulses with 1013 photons and a duration of 100 fs. Focusing this radiation to a spot some 10 μm in diameter generates intensities of up to 1016 W/cm2. Such pump intensities make feasible the investigation of photopumped XUV lasers using this radiation. We present simulations taking into account two different mechanisms generating the gain: (1) photoionization with subsequent three-body recombination, which takes advantage of the monochromaticity of the pump radiation to generate very cold electrons; (2) inner-shell ionization in which transient inversion is obtained by generating a hole in an otherwise completely filled shell. The simulations show that under appropriate conditions both mechanisms generate very high gain. However, a number of further issues must be considered, such as the propagation of the pump pulse in the medium to be pumped.

Hot electrons may significantly influence interaction of ultrashort laser pulses with solids. Accurate consideration of resonant absorption of laser energy and hot electron generation at a critical surface was achieved through the developed physical and mathematical models. A two-dimensional (2D) ray-tracing algorithm has been developed to simulate laser beam refraction and Bremsstrahlung absorption with allowance for nonlinear influence of a strong electromagnetic field. Hot electron transport was considered as a straight-line flow weakening by a friction force calculated in the approximation of the average state of ionization. Developed models were coupled with the 2D Lagrangian gas dynamic code “ATLANT” that takes into account nonlinear heat transport. The developed program has been applied to simulate irradiation of Al foils by picosecond laser double pulses. Hot electron transport and heating resulted in thin foil explosions. The transition from the exploding foil regime to the ablative one with foil thickening has been simulated and analyzed at various values of laser light intensity. In second series of calculations we have modeled the interaction of a nanosecond iodine laser with a two-layered target.

In this article, we demonstrate the generation of four phase-locked harmonic pulses separated in time using frequency-domain interferometry. The spectra present a high sensitivity to a change of the relative phase on an attosecond time scale. The spectral resolution and the control of this relative phase could be used to perform high resolution measurements.

A XUV Michelson interferometer has been developed by LIXAM/CEA/LCFIO and has been tested as a Fourier-transform spectrometer for measurement of X-ray laser line shape. The observed strong deformation of the interference fringes limited the interest of such an interferometer for plasma probing. Because the fringe deformation was coming from a distortion of the beam splitter (5 × 5 mm2 open aperture, about 150 nm thick), several parameters of the multilayer deposition used for the beam splitter fabrication have been recently optimized. The flatness has been improved from 80 nm rms obtained by using the ion beam sputtering technique, to 20 nm rms by using the magnetron sputtering technique. Over 3 × 3 mm2, the beam splitter has a flatness better than 4 nm rms.

Ultrashort pulsed hard X rays are generated by focusing an intense femtosecond laser beam onto metal targets. Kα emissions are obtained from a Cu target. Picosecond time-resolved X-ray diffraction is performed to investigate structural dynamics of laser-shocked semiconductors using the laser plasma X-ray pulses. Lattice deformation associated with shock-wave propagation is directly observed. Evolution of strain profiles inside the crystal is determined without disturbance from the time-resolved X-ray diffraction patterns.

New easy spectrally tunable backlighting schemes based on a spherically bent crystal are considered. Contrary to traditional backlighting scheme, in which the investigated objects should be placed between the backlighter and the crystal, for the considered schemes an object is placed downstream of the crystal, before the tangential or after the sagittal focus and an image of the object is recorded at the distance from the object corresponding to the needed magnification. The magnification is defined by the ratio of the distances from the sagittal focus to the detector and from the object to the sagittal focus. A ray-tracing modeling and experimental images of test meshes, obtained at incidence angles of the backlighter radiation of 10° and 22°, are presented. It is demonstrated that a simple linear transformation of the obtained astigmatic images allows reconstructing them as a stigmatic with an accuracy of 5–15%. For the spectral range around 9 Å a spatial resolution about 10 μm in a field of view of some square millimeters is achieved experimentally and confirmed by ray-tracing simulations.

Recent results on constructing of an efficient hard X-ray source using solid targets irradiated by high-contrast 200-fs laser pulses with an intensity above 1016 W/cm2 are presented. We used different solid targets with a laser- and electrochemically modified surface layer: craters, pyramidal cavities, porous silicon, gratings. Experimental data obtained confirms that using solid targets with a corrugated surface one can achieve a prominent increase both in the efficiency of hard X-ray generation (in the quanta range 2–30 keV) and in the hot electron temperature of plasma.

The mechanism of electron acceleration by intense laser pulse interacting with an underdense plasma layer is examined by one-dimensional particle-in-cell (1D-PIC) simulations. The standard dephasing limit and the electron acceleration process are discussed briefly. A new phenomenon, of short high-quality, well-collimated return relativistic electron beam with thermal energy spread, is observed in the direction opposite to laser propagation. The process of the electron beam formation, its characteristics, and the time-history in x and px space for test electrons in the beam, are analyzed and exposed clearly. Finally, an estimate for the maximum electron energy appears in a good agreement with simulation results.

The propagation of laser-generated hot electrons through matter and across narrow vacuum gaps is studied. We use the ATLAS titanium–sapphire laser of Max-Planck-Institut für Quantenoptik to irradiate aluminum and copper foils at intensities of up to 1019 W/cm2, generating electrons with temperatures in the megaelectron volt range. After propagating through the target the electrons are detected by means of visible Čerenkov radiation generated in a dielectric or hard X-rays emitted from an X-ray “fluor.” These diagnostics allow the electrons to be characterized with respect to their energy, number, and directionality. We also investigate the propagation of the hot electrons across narrow vacuum gaps, with a width ranging from 500 μm down to 50 μm. The effect of self-generated fields in preventing electrons from crossing the gap is demonstrated. Implications of these experiments with respect to fast ignitor physics, developing optics for fourth-generation light sources and X-ray lasers are indicated.

An ensemble of new techniques has been developed to study cell metabolism. These include: CO2 production monitoring, cell irradiation with soft X rays produced with a laser-plasma source, and study of oscillations in cell metabolic activity via spectral analysis of experimental records. Soft X-rays at about 0.9 keV, with a very low penetration in biological material, were chosen to produce damages at the metabolic level, without great interference with DNA activity. The use of a laser-plasma source allowed a fast deposition of high doses. Monitoring of CO2 production allowed us to measure cell metabolic response immediately after irradiation in a continuous and noninvasive way. Also a simple model was developed to calculate X-ray doses delivered to the different cell compartments following a Lambert–Bouguet–Beer law. Results obtained on Saccharomyces cerevisiae yeast cells in experiments performed at Rutherford Appleton Laboratory are presented.

The dependence of the high-order harmonic cutoff spectrum from the absolute phase of the laser pulse is here experimentally investigated. Noticeable shifts are observed. Their interpretation is proposed with a model based on the absolute-phase dependence of the trajectories of the photoelectrons that contribute to a given harmonic order.

SPARC and SPARX are two different initiatives toward an Italian Free Electron Laser (FEL) source operating in the Self Amplified Spontaneous Emission (SASE) mode, in which several national research institutions are involved. SPARC is a high gain FEL project devoted to provide a source of visible and VUV radiation while exploiting the SASE mechanism. An advanced Photo-Injector system, emittance compensating RF-gun plus a 150 MeV Linac, will inject a high quality e-beam into the undulator to generate high brilliance FEL radiation in the visible region at the fundamental wavelength, (∼500 nm). The production of flat top drive laser beams, high peak current bunches, and emittance compensation scheme will be investigated together with the generation of higher harmonic radiation in the VUV region. SPARX is the direct evolution of such a high gain SASE FEL toward the 13.5 and 1.5 nm operating wavelengths, at 2.5 GeV. To get the required value for the bunch peak current, Ipeak ≈ 2.5 kA, the “hybrid” scheme, RF-compression stage plus magnetic chicane, is analyzed and compared with the more standard double stage of magnetic compression. The two options are reviewed considering the tolerance to the drive laser pulse phase jitter.